The toolbar icons can be set to the size defined by the GTK theme, which may have detailed size control maybe, or to "very small", "small", and "large" but they will only do anything if the icon theme has those sizes and it has become common these days to provide less sizes.

Try and see if you can define GTK CSS to change the icons sizes so long as the icon theme provides a SVG icon that can be resized.

None of these are within Geany control, so it is not a bug in Geany, nor a feature that will be part of Geany.

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